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Femtosecond Magneto-Optical Pump-Probe Apparatus


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Ultrafast laser

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femtosecond laser schematic In this experiment we observe extremely fast magnetic processes by means of an optical pump-probe technique. An ultrafast Titanium-sapphire laser supplies pulses of light, less than 10-13s in duration and with wavelength tuneable in the range 700-1000 nm, at a repetition rate of 82 MHz. Each pulse is divided into two parts and the first part is used to "pump" the sample. The second is time delayed before being used to "probe" the sample at a later time. Every pair of pulses pump and probe the same process. By averaging for just 1s we collect 82 million events which leads to an excellent signal to noise ratio! The time delay can be varied by reflecting the probe beam off a mirror mounted on a translation stage, so that the sample response can be mapped out as a function of delay time.

switch schematic switch and
transmission line We use the Magneto Optical Kerr Effect to sense the instantaneous magnetic state of the sample. The sample magnetisation causes the plane of polarisation of the probe beam to be slightly rotated. Although this rotation is small we can measure the rotation to about 1 microdegree with an optical "bridge" detector that consists of a polariser and two photodiodes. We have two methods of pumping the sample. Firstly we may directly excite electrons in the surface of the sample with the optical pump pulse. Secondly we can use the optical pump pulse to trigger a magnetic field pulse by using a photoconductive switch structure. This consists of a transmission line structure deposited on a semi-insulating direct band-gap semiconductor substrate. A bias voltage is applied between the tracks of the transmission line. The substrate only conducts when the optical pump pulse creates free carriers in the gap between the tracks. At this point a current pulse is generated in the transmission line. The magnetic field associated with the current is used to "pump" the sample that is overlaid on the transmission line. The current profile can be checked either by attaching an oscilloscope to the transmission line, or by using the probe pulse to divert current into a third Au track and so generate a current autocorrelation curve.

                                                                                                                                                                                                                                                                       

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